The Cantilever-based NOSE

H.P. Langa,b, M.K. Ballera,b, F.M. Battistonb, J. Fritz a,b, R. Bergerc, J.-P. Ramseyerb
P. Fornarob, E. Meyerb, H.-J. Güntherodtb, J. Bruggera, U. Drechslera, H. Rothuizena,
M. Desponta, P. Vettigera, Ch. Gerbera, J.K. Gimzewskia
 
aIBM Research Division, Zurich Research Laboratory
Säumerstrasse 4, CH-8803 Rüschlikon (Switzerland)
bInstitute of Physics, University of Basel
Klingelbergstrasse 82, CH-4056 Basel (Switzerland)
cIBM SSD GmbH,
Dept. 4119, Hechtsheimer Strasse 2, D-55131 Mainz (Germany)
Tel: ++41 1 724 8929

We present a novel chemical sensor based on a microfabricated array of silicon cantilevers. Individual cantilevers are sensitized for the detection of analytes using metal coatings, self-assembled monolayers or polymers.
Analyte molecules chemisorbing or physisorbing on the cantilever coating and chemical reactions produce a change in interfacial stress between adsorbed analyte molecule layer and cantilever surface. This leads to a nanomechanical response of the cantilever, i.e. bending
Combining various sensors within an array creates a device which can be employed as a Nanomechanical Olfactory Sensor (NOSE). Cantilever bending is detected using a time-multiplexed optical beam-deflection technique. From magnitude and temporal evolution of the bending, quantitative information on analyte species and concentration is derived. Using an automatized gas handling system, we demonstrate detection of ethene with such a nanomechanical nose.
Other analytes, such as water and various primary alcohols can be investigated by conducting the carrier gas through a vessel filled with a few ul of liquid analyte by means of the gas handling system. Employing polymer coatings as cantilever sensor layers we can observe diffusion of analyte-saturated carrier gas into the polymer layer by tracking the bending of cantilevers.
Applying principal component analysis (PCA) chemical analytes can be distinguished by different temporal evolution of sensor responses.